Oscillatory cluster patterns in a homogeneous chemical system with global
feedback
Vanag VK, Yang LF, Dolnik M, Zhabotinsky AM, Epstein IR
NATURE
406 (6794): 389-391 JUL 27 2000
Abstract:
Oscillatory clusters are sets of domains in which nearly all elements
in a given domain oscillate with the same amplitude and
phase(1-4). They play an important role in understanding coupled neuron
systems(5-8). In the simplest case, a system consists of
two clusters that oscillate in antiphase and can each occupy multiple
fixed spatial domains. Examples of cluster behaviour in
extended chemical systems are rare, but have been shown to resemble
standing waves(9-13), except that they lack a
characteristic wavelength. Here we report the observation of so-called
'localized clusters'-periodic antiphase oscillations in one
part of the medium, while the remainder appears uniform-in the Belousov-Zhabotinsky
reaction-diffusion system with
photochemical global feedback. We also observe standing clusters with
fixed spatial domains that oscillate periodically in time and
occupy the entire medium, and irregular clusters with no periodicity
in either space or time, with standing clusters transforming into
irregular clusters and then into localized clusters as the strength
of the global negative feedback is gradually increased. By
incorporating the effects of global feedback into a model of the reaction,
we are able to simulate successfully the experimental
data.